I've used Partition Majic for years. Good choice. No experience with the other, so no opinion.
However, consider another method. It IS more hassle, but you'll have a better system when done.
Best practices suggests installing only system-related software (OS, AntiVirus, hardware drivers, etc.) on the C: partition. This partition also should not be over 8-12 GB. All other software (Office, games, etc.) should be installed in a different partition, which can be as large as you want or need. Have a third partition (the really large one) for non-program files, such as pictures, music, videos, etc.
To reinstall the software you'll likely need any license keys that came with them, as well as the CDs.
Shrink the really large partition by 50-70GB (or more). Take that 60GB (or so) partition and format it, preferably with NTFS. Install ALL future programs into it.
Also, consider uninstalling any non-system-related software (see above) from C: and reinstalling it to the new partition. Once done, you should defrag the C: partition then shrink it (if possible - Partition Magic can do this) to some smaller size. Add that extra space to your new Game (or whatever) partition.
Defrag the partitions once you're done.
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